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Polarized Raman Study of 2-dimensional Layered Gallium Selenide

초록/요약

Gallium Selenide (GaSe) is a layered semiconductor composed of post-transition metal Gallium (Ga) and chalcogen Selenidum (Se). It can be used in a photodevice thanks to high photoresponsivity and external quantum efficiency. [1,2] We investigated layered GaSe by polarized Raman spectroscopy from monolayer to bulk. The A1g1 mode blueshifts with increasing thickness while other peaks do not change much. We also observed low frequency shear modes coming from inter-layer vibrations in the range of 5-25 cm-1. The layer number of GaSe was determined by the position of the shear modes and atomic force microscopy. We also found domains with different stacking orders even in same-thickness flakes. We measured 3-layer GaSe samples in particular. We found several types of low-frequency spectra that correspond to different stacking orders.

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